Abstract
Time-of-flight secondary ion mass spectrometry (ToF-SIMS) chemical mapping was used to investigate the order of deposition of natural latent fingerprints and laser printed ink on paper. This feasibility study shows that sodium, potassium and C3H5 positive ions were particularly abundant endogenous components of the natural fingerprints and also present in the paper examined, but were mostly absent in the laser printed ink. Mapping of these ions enables the observation of friction ridges from latent prints on the ink surface, only when a fingerprint was deposited above the layer of ink. As a demonstration of proof of concept, blind testing of 21 samples from three donors resulted in a 100% success rate. The sensitivity of this technique was investigated within this trial through the examination of up to fifth depletion fingerprints and ageing of up to 28days. Migration of fingerprint and paper components to the ink surface, although observed with increased ageing time, was not found to compromise determination of the deposition sequence.
| Original language | English |
|---|---|
| Pages (from-to) | 2-7 |
| Number of pages | 6 |
| Journal | Science and Justice |
| Volume | 53 |
| Issue number | 1 |
| Early online date | 2 Jul 2012 |
| DOIs | |
| Publication status | Published - Mar 2013 |
| Externally published | Yes |
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Determining the order of deposition of natural latent fingerprints and laser printed ink using chemical mapping with secondary ion mass spectrometry. / Attard Montalto, Nicola; Ojeda, Jesús J.; Jones, Benjamin J.
In: Science and Justice, Vol. 53, No. 1, 03.2013, p. 2-7.Research output: Contribution to journal › Article
TY - JOUR
T1 - Determining the order of deposition of natural latent fingerprints and laser printed ink using chemical mapping with secondary ion mass spectrometry
AU - Attard Montalto, Nicola
AU - Ojeda, Jesús J.
AU - Jones, Benjamin J.
PY - 2013/3
Y1 - 2013/3
N2 - Time-of-flight secondary ion mass spectrometry (ToF-SIMS) chemical mapping was used to investigate the order of deposition of natural latent fingerprints and laser printed ink on paper. This feasibility study shows that sodium, potassium and C3H5 positive ions were particularly abundant endogenous components of the natural fingerprints and also present in the paper examined, but were mostly absent in the laser printed ink. Mapping of these ions enables the observation of friction ridges from latent prints on the ink surface, only when a fingerprint was deposited above the layer of ink. As a demonstration of proof of concept, blind testing of 21 samples from three donors resulted in a 100% success rate. The sensitivity of this technique was investigated within this trial through the examination of up to fifth depletion fingerprints and ageing of up to 28days. Migration of fingerprint and paper components to the ink surface, although observed with increased ageing time, was not found to compromise determination of the deposition sequence.
AB - Time-of-flight secondary ion mass spectrometry (ToF-SIMS) chemical mapping was used to investigate the order of deposition of natural latent fingerprints and laser printed ink on paper. This feasibility study shows that sodium, potassium and C3H5 positive ions were particularly abundant endogenous components of the natural fingerprints and also present in the paper examined, but were mostly absent in the laser printed ink. Mapping of these ions enables the observation of friction ridges from latent prints on the ink surface, only when a fingerprint was deposited above the layer of ink. As a demonstration of proof of concept, blind testing of 21 samples from three donors resulted in a 100% success rate. The sensitivity of this technique was investigated within this trial through the examination of up to fifth depletion fingerprints and ageing of up to 28days. Migration of fingerprint and paper components to the ink surface, although observed with increased ageing time, was not found to compromise determination of the deposition sequence.
U2 - 10.1016/j.scijus.2012.05.007
DO - 10.1016/j.scijus.2012.05.007
M3 - Article
C2 - 23380055
AN - SCOPUS:84873107422
VL - 53
SP - 2
EP - 7
JO - Science and Justice - Journal of the Forensic Science Society
JF - Science and Justice - Journal of the Forensic Science Society
SN - 1355-0306
IS - 1
ER -